<i>Ab initio</i> coupled-cluster calculations of ground and dipole excited states in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mmultiscripts><mml:mi>He</mml:mi><mml:mprescripts /><mml:none /><mml:mn>8</mml:mn></mml:mmultiscripts></mml:math>
نویسندگان
چکیده
We perform coupled-cluster calculations of ground- and dipole excited-state properties the 8He halo nucleus with nucleon-nucleon three-nucleon interactions from chiral effective field theory, both without explicit delta degrees freedom. By increasing precision in our via inclusion leading order three-particle three-hole excitations cluster operator, we obtain a ground-state energy charge radius that are consistent experiment, albeit slight under-binding. also investigate excited states induced by electric operator present discussion on Thomas-Reiche-Kuhn sum rules. Finally, compute polarizability, providing theoretical benchmark for future experimental determinations will study this exotic nucleus.
منابع مشابه
Coupled-cluster calculations for the ground and excited states of the spin-half XXZ model.
The coupled-cluster method is applied to the spin-1/2 antiferromagnetic XXZ model on a square lattice by employing an approximation which contains two-body long-range correlations and high-order four-body local correlations. Improvement is found for the ground-state energy, the sublattice magnetization and the critical anisotropy when comparing with the approximation including the two-body corr...
متن کاملCoupled Cluster Calculations of the Ground and Excited Electronic States Using Two- and Four- Component Relativistic Spinors
The coupled cluster based linear response theory which is applicable to the direct calculation of atomic and molecular properties are presented and applied to compute the ionization potentials and excitation energies of light and moderately heavy atoms. The effect of electron correlation on the ground and excited states is studied using Hartree-Fock, Dirac-Fock and approximate two-component rel...
متن کاملQuantum Monte Carlo Calculations for Ground and Excited States
A brief overview of the diffusion quantum Monte Carlo method is given. We illustrate the application to ground-state calculations by a study of the relative stability of carbon clusters near the crossover to fullerene stability, thereby determining the smallest stable fullerene. The application to excited states is illustrated via a study of excitonic states in small hydrogenated silicon cluste...
متن کاملCoupled-cluster with active space selected higher amplitudes: performance of seminatural orbitals for ground and excited state calculations.
The active space approach for coupled-cluster models is generalized using the general active space concept and implemented in a string-based general coupled-cluster code. Particular attention is devoted to the choice of orbitals on which the subspace division is based. Seminatural orbitals are proposed for that purpose. These orbitals are obtained by diagonalizing only the hole-hole and particl...
متن کاملProton Affinities of Didehydroporphyrin and Subporphyrin in Ground and Excited States Obtained by Quantum Chemical Calculations*
Quantum-chemical calculations were used to investigate molecular and electronic properties of porphyrin and subporphyrin. Their basicities were estimated in ground and excited states. It was found that multiple proton nitrogen lone-pair coordination plays an important role in acid/base properties of the studied molecules. Lone pair-lone pair interactions in didehydroporphyrin and energetic stab...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
ژورنال
عنوان ژورنال: Physical Review C
سال: 2022
ISSN: ['2470-0002', '2469-9985', '2469-9993']
DOI: https://doi.org/10.1103/physrevc.105.034313